EPITAXIAL GROWTH OF FCC Ti FILMS ON Al(001) SURFACES

Adli A. Saleh, V. Shutthanandan, N.R. Shivaparan and R.J. Smith,
Department of Physics, Montana State University, Bozeman, Montana 59717*

T. T. Tran and S. A. Chambers
Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory,
Richland, Washington 99352**


High-energy ion scattering (HEIS), x-ray photoelectron spectroscopy (XPS), and x-ray photoelectron diffraction (XPD) were used to study the growth of thin Ti films on Al(001) surfaces. The Al surface peak area in the backscattered ion spectrum of MeV He+ ions, incident along the [00 -1] direction, was used to monitor the atomic structure of the Ti films during growth. An initial decrease in the area was observed indicating epitaxial film growth. This decrease continued up to a critical film thickness of about 5.5 monolayers, after which point the structure of the film changed. Titanium films, 3, 5, and 9 monolayers thick, were characterized using XPD in the same chamber. Both the HEIS and XPD results show that the Ti films grow with an fcc structure on Al(001). A tetragonal distortion of 2.4 % in the fcc Ti film was measured using ions incident along the [10 -1] direction. Although there is a general similarity of fcc Ti growth on both Al(001) and Al(110), the submonolayer growth regime does show differences for the two surfaces.
*Work supported by NSF Grant No. DMR-9409205 and NASA EPSCoR Grant NCCW-0058
**Work at PNL supported under Contract DE-AC06-76RLO 1830

Physical Review B56, 9841 (1997)

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